| — | Zero Day | George Mullen |
| — | De Niro, New York | Himself |
| — | After Exile | Ted Delaney |
| — | Untitled De Niro/Ramirez/Jakubowicz Project | G.B. |
| 2025 | Tin Soldier | Emmanuel Ashburn |
| 2025 | Alto Knights | Vito Genovese / Frank Costello |
| 2024 | How to Rob a Bank | Neil McCauley (archive footage) |
| 2024 | Ezra | Stan Bernal |
| 2024 | #LoveArmy : Où es-tu Jérôme ? | Lui-même (Archive) |
| 2023 | Killers of the Flower Moon | William Hale |
| 2023 | About My Father | Salvo |
| 2023 | Sly | Self (archive footage) (uncredited) |
| 2023 | Nothing | Vincent |
| 2023 | 100 Years of Warner Bros. | Self |
| 2023 | Albert Brooks: Defending My Life | Self |
| 2023 | Hot Potato: The Story of The Wiggles | Self (archive footage) (uncredited) |
| 2023 | Martin Scorsese, l'Italo-Américain | Self |
| 2023 | Robert De Niro: Hiding in the Spotlight | Self - Portrait Subject (archive footage) |
| 2023 | The Randall Scandal: Love, Loathing, and Vanderpump | Self (archive footage) (uncredited) |
| 2022 | Amsterdam | General Gil Dillenbeck |
| 2022 | Savage Salvation | Sheriff Church |
| 2022 | Sergio Leone: The Italian Who Invented America | Self |
| 2022 | Becoming Al Pacino | Self (archive footage) |
| 2022 | Prisoners of Our Own History: The First Four Films of Roland Joffé | Self (archive footage) |
| 2022 | The Past Goes Fast | Self |
| 2021 | Mr. Saturday Night | |
| 2021 | Quentin Tarantino: From a Movie Buff to a Hollywood Legend | Video footage |
| 2020 | The War with Grandpa | Ed |
| 2020 | The Comeback Trail | Max Barber |
| 2020 | Crazy, Not Insane | Self (archive footage) |
| 2020 | Father of the Bride Part 3 (ish) | James |
| 2020 | Some Good News | Weatherman |
| 2020 | Charles Bronson: The Spirit of Masculinity | Self (archive footage) |
| 2020 | 537 Votes | Self (archive footage) |
| 2020 | Making 'The Irishman' | Self |
| 2020 | The Collaboration Of A Lifetime: Scorsese’s Epic The Irishman | Self |
| 2020 | A Shot In The Dark | himself |
| 2020 | The Bee | Neil McCauley (archive footage) |
| 2019 | Joker | Murray Franklin |
| 2019 | The Irishman | Frank Sheeran |
| 2019 | QT8: The First Eight | Self (archive footage) |
| 2019 | The Irishman: In Conversation | Self |
| 2019 | Comedy Central Roast of Alec Baldwin | Self |
| 2019 | I Am Durán | Himself |
| 2018 | Breslin and Hamill: Deadline Artists | Self |
| 2018 | The Alec Baldwin Show | Self |
| 2017 | The Wizard of Lies | Bernie Madoff |
| 2017 | Jim Norton: Mouthful of Shame | Self (uncredited) |
| 2017 | The Words That Built America | Self - Reader - Declaration of Independence |
| 2017 | Alec Baldwin: One Night Only | Himself |
| 2016 | Dirty Grandpa | Dick Kelly |
| 2016 | Hands of Stone | Ray Arcel |
| 2016 | The Comedian | Jackie Burke |
| 2016 | Full Frontal with Samantha Bee | Self |
| 2016 | Tony Bennett Celebrates 90 | Self |
| 2016 | I Am JFK Jr. | Self |
| 2016 | National Museum of African American History and Culture Grand Opening Ceremony | Self |
| 2015 | The Intern | Ben Whitaker |
| 2015 | Joy | Rudy |
| 2015 | Heist | The Pope |
| 2015 | The Late Show with Stephen Colbert | Self |
| 2015 | The Late Show with Stephen Colbert | |
| 2015 | The Audition | Robert De Niro |
| 2015 | Ellis | |
| 2015 | Peggy Guggenheim: Art Addict | Himself |
| 2015 | Close Up with The Hollywood Reporter | Self |
| 2015 | Scorsese's GoodFellas | Self |
| 2015 | Saturday Night Live: 40th Anniversary Special | Self |
| 2014 | The Bag Man | Dragna |
| 2014 | The Tonight Show Starring Jimmy Fallon | Self |
| 2014 | Late Night with Seth Meyers | Self |
| 2014 | The Man Who Saved the World | Self |
| 2014 | Remembering the Artist: Robert De Niro, Sr. | Himself |
| 2014 | Don Rickles: One Night Only | Self |
| 2014 | Robin Williams Remembered | Self |
| 2014 | Inside Rupert Pupkin | Self (archive footage) |
| 2013 | American Hustle | Victor Tellegio (uncredited) |
| 2013 | The Family | Fred Blake / Giovanni Manzoni |
| 2013 | Last Vegas | Patrick 'Paddy' Connors |
| 2013 | Grudge Match | Billy 'The Kid' McDonnen |
| 2013 | The Big Wedding | Don Griffin |
| 2013 | Killing Season | Benjamin Ford |
| 2013 | David Blaine: Real or Magic | Self |
| 2013 | Trespassing Bergman | Self |
| 2013 | Miracle Rising: South Africa | Self |
| 2012 | Silver Linings Playbook | Pat Solatano Sr. |
| 2012 | Red Lights | Simon Silver |
| 2012 | Being Flynn | Jonathan Flynn |
| 2012 | Freelancers | Sarcone |
| 2012 | Final Cut: Ladies and Gentlemen | (archive footage) |
| 2012 | Casting By | Self |
| 2012 | Bergmans video | Self |
| 2012 | Close Up | Self (archive footage) |
| 2011 | Limitless | Carl Van Loon |
| 2011 | New Year's Eve | Stan Harris |
| 2011 | Killer Elite | Hunter |
| 2011 | Ages of Love | Adrian |
| 2011 | Corman's World | Self - Actor |
| 2011 | 9/11: 10 Years Later | Host |
| 2011 | Behind Bars: The Making of Stone | Self |
| 2011 | Marty and Bobby | Self |
| 2010 | Machete | Senator John McLaughlin |
| 2010 | Little Fockers | Jack Byrnes |
| 2010 | Stone | Jack |
| 2010 | Sesame Street: 40 Years of Sunny Days | Self (uncredited) (archive footage) |
| 2009 | Everybody's Fine | Frank Goode |
| 2009 | The Cleveland Show | |
| 2009 | Late Night with Jimmy Fallon | Self |
| 2009 | I Knew It Was You: Rediscovering John Cazale | Self |
| 2009 | SNL Presents: A Very Gilly Christmas | |
| 2008 | Righteous Kill | Detective Tom 'Turk' Cowan |
| 2008 | What Just Happened | Ben |
| 2008 | The Beaches of Agnès | Self (archive footage) |
| 2007 | Stardust | Captain Shakespeare |
| 2007 | The Graham Norton Show | Self - Guest |
| 2007 | The Graham Norton Show | Self |
| 2007 | Mr. Warmth: The Don Rickles Project | Self |
| 2007 | Le Cirque: A Table in Heaven | Self |
| 2007 | God's Lonely Man | Self - Archive Footage |
| 2007 | Influence And Appreciation: A Martin Scorsese Tribute | Self |
| 2007 | Making Casino | Self |
| 2006 | Arthur and the Invisibles | King (voice) |
| 2006 | The Good Shepherd | Bill Sullivan |
| 2006 | 30 Rock | Robert De Niro |
| 2006 | Tony Bennett: An American Classic | Self - Speaker |
| 2005 | Hide and Seek | David Callaway |
| 2005 | Extras | Robert De Niro |
| 2005 | Club Oscar | Don Lino (voice) |
| 2005 | The Reichen Show | Self |
| 2005 | The Making of 'Heat' | Self |
| 2005 | Raging Bull: Before the Fight | Self |
| 2005 | Raging Bull: Inside the Ring | Self (archive footage) |
| 2005 | Pacino and De Niro: The Conversation | Self |
| 2005 | Raging Bull: Outside the Ring | Self |
| 2005 | Raging Bull: After the Fight | Self (archive footage) |
| 2005 | The 'New York, New York' Stories | Self (archive footage) |
| 2004 | Shark Tale | Don Lino (voice) |
| 2004 | Meet the Fockers | Jack Byrnes |
| 2004 | Fahrenheit 9/11 | Self (archive footage) (uncredited) |
| 2004 | Godsend | Richard Wells |
| 2004 | The Bridge of San Luis Rey | Archbishop of Peru |
| 2004 | The 50 Worst Movies Ever Made | Jon Rubin (archive footage) |
| 2004 | Ronin: Filming in the Fast Lane | Self |
| 2004 | Getting Made: The Making of 'GoodFellas' | Self |
| 2003 | Real Time with Bill Maher | Self |
| 2003 | Jimmy Kimmel Live! | Self - Guest |
| 2003 | Comedy Central Roasts | Self |
| 2002 | Analyze That | Paul Vitti |
| 2002 | Showtime | Det. Mitch Preston |
| 2002 | City by the Sea | Vincent LaMarca |
| 2002 | 9/11 | Himself |
| 2002 | Jackie Brown: How It Went Down | Self |
| 2002 | A Shot at the Top: The Making of 'The King of Comedy' | Self (archive footage) |
| 2001 | The Score | Nick Wells |
| 2001 | 15 Minutes | Eddie Flemming |
| 2001 | The Making of 'Cape Fear' | Self |
| 2001 | The Concert for New York City | Self |
| 2000 | Meet the Parents | Jack Byrnes |
| 2000 | Men of Honor | Master Chief Leslie W. Sunday ('Billy') |
| 2000 | The Adventures of Rocky & Bullwinkle | Fearless Leader |
| 1999 | Analyze This | Paul Vitti |
| 1999 | Flawless | Walt Koontz |
| 1999 | Making 'Taxi Driver' | Self |
| 1998 | Ronin | Sam |
| 1998 | Great Expectations | Prisoner / Lustig |
| 1998 | Lenny Bruce: Swear to Tell the Truth | Himself / Narrator (voice) |
| 1998 | Junket Whore | Self |
| 1997 | Jackie Brown | Louis Gara |
| 1997 | Cop Land | Lt. Moe Tilden |
| 1997 | Wag the Dog | Conrad Brean |
| 1997 | The View | Self |
| 1996 | Sleepers | Father Bobby |
| 1996 | The Fan | Gil Renard |
| 1996 | Marvin's Room | Wallace "Wally" Carter |
| 1996 | The Daily Show | Self |
| 1995 | Heat | Neil McCauley |
| 1995 | Casino | Sam 'Ace' Rothstein |
| 1995 | One Hundred and One Nights | The Husband of The Star-Fantasy on a Cruise |
| 1995 | Ennio Morricone | Self (archive footage) |
| 1994 | Mary Shelley's Frankenstein | The Creature / Sharp Featured Man |
| 1994 | Inside the Actors Studio | Self |
| 1994 | It's Alive: The True Story of Frankenstein | Self |
| 1994 | You Talkin' to Me? | Self |
| 1993 | A Bronx Tale | Lorenzo Anello |
| 1993 | This Boy's Life | Dwight Hansen |
| 1993 | Mad Dog and Glory | Wayne "Mad Dog" Dobie |
| 1993 | Aretha Franklin: Duets | Self |
| 1992 | The Tonight Show with Jay Leno | |
| 1992 | Night and the City | Harry Fabian |
| 1992 | Mistress | Evan M. Wright |
| 1991 | Cape Fear | Max Cady |
| 1991 | Backdraft | Donald Rimgale |
| 1991 | Guilty by Suspicion | David Merrill |
| 1990 | GoodFellas | James Conway |
| 1990 | Awakenings | Leonard Lowe |
| 1990 | Stanley & Iris | Stanley Everett Cox |
| 1990 | The Godfather Family: A Look Inside | Self |
| 1990 | Martin Scorsese Directs | Self |
| 1990 | Hollywood Mavericks | Self |
| 1989 | We're No Angels | Ned |
| 1989 | Jacknife | Joseph 'Jacknife' Megessey |
| 1988 | Midnight Run | Jack Walsh |
| 1988 | LIVE with Kelly and Mark | |
| 1988 | Hello Actors Studio | Self |
| 1987 | The Untouchables | Al Capone |
| 1987 | Angel Heart | Louis Cyphre |
| 1987 | Dear America: Letters Home from Vietnam | Great Sewer (voice) |
| 1986 | The Mission | Rodrigo Mendoza |
| 1985 | Brazil | Harry Tuttle |
| 1985 | Night of 100 Stars II | Self |
| 1984 | Once Upon a Time in America | David 'Noodles' Aaronson |
| 1984 | Falling in Love | Frank Raftis |
| 1982 | The King of Comedy | Rupert Pupkin |
| 1982 | Elia Kazan: An Outsider | Self |
| 1982 | Night of 100 Stars | Self |
| 1981 | True Confessions | Father Des Spellacy |
| 1981 | The Godfather 1901–1959: The Complete Epic | Young Vito Corleone |
| 1980 | Raging Bull | Jake LaMotta |
| 1979 | The Swap | Sam Nicoletti (archive footage) |
| 1978 | The Deer Hunter | Michael Vronsky |
| 1978 | Movies Are My Life | Self |
| 1977 | New York, New York | Jimmy Doyle |
| 1977 | Mario Puzo's The Godfather: The Complete Novel for Television | Young Vito Corleone |
| 1977 | Auf los geht's los | Self |
| 1976 | Taxi Driver | Travis Bickle |
| 1976 | 1900 | Alfredo Berlinghieri |
| 1976 | The Last Tycoon | Monroe Stahr |
| 1976 | The Cinema According to Bertolucci | Self |
| 1975 | Saturday Night Live | Self - Host |
| 1975 | Saturday Night Live | Self |
| 1975 | Saturday Night Live | Self - Cameo (uncredited) |
| 1975 | Saturday Night Live | Boss |
| 1975 | Abicinema | Self |
| 1974 | The Godfather Part II | Vito Corleone |
| 1973 | Mean Streets | John 'Johnny Boy' Civello |
| 1973 | Bang the Drum Slowly | Bruce Pearson |
| 1971 | Born to Win | Danny |
| 1971 | The Gang That Couldn't Shoot Straight | Mario |
| 1971 | Jennifer on My Mind | Mardigian |
| 1970 | Hi, Mom! | Jon Rubin |
| 1970 | Bloody Mama | Lloyd Barker |
| 1969 | The Wedding Party | Cecil |
| 1969 | Sam's Song | Sam Nicoletti |
| 1968 | Greetings | Jon Rubin |
| 1968 | Young Wolves | Un hippie chez Popov (uncredited) |
| 1966 | Goldene Kamera Verleihung | Self |
| 1965 | Three Rooms in Manhattan | Client at the Diner (uncredited) |
| 1953 | The Oscars | Self |
| 1944 | Golden Globe Awards | Self - Nominee |
